George Clooney did not make any such claims about Meghan Markle in the documentary "Always at the Carlyle." The documentary, which was released in 2018, features interviews with a number of celebrities and hotel staff about their experiences at the Carlyle, a luxury hotel in New York City. Clooney is one of the interviewees, and he does not mention Markle at all.
The claim that Clooney made these claims about Markle appears to have originated from a blog post published in January 2023. The blog post, which is no longer available online, claimed that Clooney had said that Markle was "bossy" and "made noise until 5 AM" during her stay at the Carlyle. However, there is no evidence to support these claims.
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The blog post also claimed that Clooney's comments were made in the documentary "Always at the Carlyle." However, as mentioned above, Clooney does not mention Markle in the documentary.
It is possible that the blog post was simply mistaken about what Clooney said. It is also possible that the blog post was intentionally spreading false information about Markle. Either way, there is no evidence to support the claim that Clooney made any negative comments about Markle in the documentary "Always at the Carlyle."